No, even if you successfully achieve a 51% attack, you can't spend coins from arbitrary wallets.
When you have 51% of mining power, you can do a lot of nasty things(like stopping confirming transaction at all), but not spend someone else's bitcoins.
The double spend attack works by convincing the other party that the transaction has completed (so they release whatever escrow is in place) and then replacing the blockchain.
(But a botnet infection could watch for wallets on a computer and cause the coins in the wallet to be spent)