I've thoroughly enjoyed using ImGui for tooling around image processing, computational geometry, a bunch of 3D projection stuff. The fact that it's based on OpenGL or Vulkan or whatever backend you want is a big win for this kind of work. I can just take a bunch of pixels, throw them into a texture, and render some quads with those textures painted on them after going through some 2D transformations or 3D projection/transformation. It's quite beautiful for all of this. ImPlot for doing basic data plotting and the built-in ImGui widgets for controlling the whole thing.
I have otherwise mostly given up on making GUI applications because I simply don't have time to pick up a bunch of UI toolkits for all the different platforms, pulling a massive dependency into my project and requiring constant maintenance to keep the program working.
It can be a bit wonky though, I regularly spot UI/UX decisions that seem to map more closely to what the developer is doing under the hood, or their own mental model of the problem, than what one might consider to be an intuitive way of interacting with the system.
This isn't to say a tool for non-engineers should have animations to make it useful. ImAnim should probably be used sparingly, if at all.
If you need the features of a full GUI toolkit, then by all means use Qt or wxWidgets etc, but that's a very big jump in project complexity.
But "development/debug tools" is actually just a subset of professional or industrial utility applications where user count is low and support is on the extremes (either "capable self-support" or "Yes, Bob, of course we'll add that for you").
And in those utility applications, you probably don't need the noisy toy animations associated with modern consumer software, but animated data representations can be really valuable.
On one hand I agree. On the other: where are these high performance real-time GUI kits these days? If it came down to IMGUI or shoving Electron into my app...
It is popular mostly because all alternatives are really bad, if "all" you want is a functional GUI to deliver some developer tool. Qt means you have to dive really deep into a C++ project. The web technologies are all far too heavy and complex and you don't really any of the power. There also are many other alternatives, none of them really do what ImGui does.