We do population level correlation studies because sometimes a double blind study is unethical, and double blind studies is the bar for establishing causation in the medical community. We cannot give one person randomly worse air to breath, and even if it were experimentally feasible it would be ethically impossible because there is strong suspicion we would be harming the subjects.
Let’s discuss the actual data. The dose dependent result that was found is an indicator of a strong relationship. There is a clear potential mechanism of action (Air -> Lungs -> Bloodstream -> Brain). This isn’t a controversial result in the literature, it’s more evidence for what we already know —- air pollution is very bad.