Recharging it isn't that simple
We use zeolite as a water scavenger in high vacuum systems, it's tremendously good at grabbing onto water BUT because it's so porous and very low thermal conductivity it's a real pain to heat it enough to get all the water out again. We have a heater resistor at the bottom of a small can of this and the top of the pellets a few cm away is cool enough to touch. You might do better with a microwave system but then the inefficiencies are going to hurt.
Why not use one of the many phase change salt solutions that are also used for rechargeable heater packs?