Anecdata of one: In my most recent (~5-6 years ago) TH phase, I listened to all the albums multiple times (one nice thing about streaming services) but the ones I kept coming back to were 'Fear of Music', 'Remain in Light', and, thirdly, 'Speaking in Tongues.' For me it's a coin-flip between FoM and RiL as their best album front-to-back.
Hoping to catch the movie while it's playing again.