I agree 100%. Originally land taxes were conceived as a correction for a more subtle bit of economic inequality: productivity of fields.
In today's world, where access to a city can dramatically change one's earning potential far far more, they are even more relevant.
The issue is both about the scarcity of access to a resource, such as the economy of a city, but also about where that resource comes from. With urban land, that resource is not the product of the individual land owner, but rather all the other land owners that made the city so prosperous and with so much opportunity.