Bucharest was fine. The lack of decor started to wear on me after a while. Cool thing about Romania is that you can rent pretty easily and leave with one month's notice even if you signed a one year lease. A decent 400 SQ ft studio in Bucharest or Cluj (the most expensive cities) won't be more than $350 a month.
I'd explore all these, may be do a few months stay in each city, that would be really cool experience you could tell stories about.
Btw if you go further east check out Chernivtsi, it’s a hidden gem in the East Carpathian mountains.
Language wise, most people under 30 had some basic English, I spoke almost no Serbian at all but still managed to get by at stores and restaurants. Internet is cheap and widely available.