We use Qt heavily at Starsky Robotics. We initially used it because it has tight integration with ROS via RQT [1], but I'm pretty impressed with the framework in general. Lots of great tools out of the box, QtCreator is awesome and once you get the right signal/slot model in your head everything is a breeze. Plus getting to prototyping in python is always fast!
For our use case, relative speed of the GUI isn't a factor. We've considered moving to electron just for ease of development, but python is winning out.