This guy lays out most of the obstacles with the process in a very short comment: 1. Maintain consistent depth of field between two cameras by using separate Neutral Density filters for each camera 2. Spend time tweaking your luma keys for each video stream.
People that work on lighting crews should be getting nervous right about now.
I think that most of the magic in this technique is in the luma keys. (duh...)
And you are right, this video (and the other one on that vimeo account) is better mostly due to process/skill and not due to equipment used. One could argue about HDR though, since it's only a technique to widen the range of possibilities within compositing. How one utilizes those can be viewed as artistic direction. I also dislike masks with visible feathering, as shown in most HDR stuff out there.