What about using zip bombs?
https://maurycyz.com/misc/the_cost_of_trash/#:~:text=throw%2...
Otherwise you can also chain compression methods like: "Content-Encoding: gzip gzip".
With toxic AI scrapers like Perplexity moving more and more to headless web browsers to bypass bot blocks, I think a brotli bomb (100GB of \0 can be compressed to about 78KiB with Brotli) would be quite effective.
I have a web crawler and I have both scraping byte limit and timeout, so zip bombs dont bother me much.
https://github.com/rumca-js/crawler-buddy
I think garbage blabber would be more effective.