The short answer is that the best value is a used RTX 3090 (the long answer being, naturally, it depends). Most of the time, the bottleneck for running LLMs on consumer grade equipment is memory and memory bandwidth. A 3090 has 24GB of VRAM, while a 5080 only has 16GB of VRAM. For models that can fit inside 16GB of VRAM, the 5080 will certainly be faster than the 3090, but the 3090 can run models that simply won't fit on a 5080. You can offload part of the model onto the CPU and system RAM, but running a model on a desktop CPU is an enormous drag, even when only partially offloaded.
Obviously an RTX 5090 with 32GB of VRAM is even better, but they cost around $2000, if you can find one.
What's interesting about this Strix Halo system is that it has 128GB of RAM that is accessible (or mostly accessible) to the CPU/GPU/APU. This means that you can run much larger models on this system than you possibly could on a 3090, or even a 5090. The performance tests tend to show that the Strix Halo's memory bandwidth is a significant bottleneck though. This system might be the most affordable way of running 100GB+ models, but it won't be fast.