I didn't know of that paper, and thought the title was a riff on Karpathy's Unreasonable Effectiveness of RNNs in 2015[1]. Even if my thinking is correct, as it very well might be given the connection RNNs->LLMs, Karpathy might have himself made his title a play on Wigner's (though he doesn't say so).

[1] https://karpathy.github.io/2015/05/21/rnn-effectiveness/