From my testing on clocks on the Pi 5, it looks like the default clock of 2.4 GHz is pretty close to the sweet spot for this chip (BCM2712), and you burn a lot of power for small incremental gains after that[1]. (Which you seem to also show with the 3.3 GHz overclock!).
I also spoke to one of the Pi engineers about the chip behavior at higher clocks, and he suggested unlike some chips, this chip might run more stably at higher temperatures (like 50-60°C) rather than 'as cold as you can get it'. So that poses some challenges since most cooling solutions aren't tuned for 'keep a temperature' but instead 'get it as cold as possible', without a lot of manual tweaking.
[1] https://www.jeffgeerling.com/blog/2023/overclocking-and-unde...