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Weirdly Goldeneye did have a control layout where you could move with one joystick and aim with the other using 2 controllers: https://www.youtube.com/watch?v=dZaEpugk3hY

That's how I played, and while the N64 joysticks aren't very good, it was alright. The much bigger problem was lag.

Yeah, it's awesome as you can set this up relatively easily with EmuDeck and play it with the two sticks on the Steam Deck.