The TMS9900 was made in I²L bipolar technology, not MOS. Texas Instruments also had a 4 wide bitslice using the same fabrication process.
TMS9900, which was 16-bit CPU in a big 64-pin package (like that used later by Motorola MC68000) was certainly made in an NMOS technology.
See e.g. Wikipedia:
https://en.wikipedia.org/wiki/TMS9900
There is no doubt about this because TMS9900 required -5 V (for substrate bias), +5 V and +12 V (for enhancement MOS load transistors), like all early NMOS ICs, e.g. Intel 8080. No bipolar technology would have needed such power supplies.
The later TMS9995 was also made in an NMOS technology, but in a more modern variant with depletion transistor loads, which required only a single +5 V power supply, like Zilog Z80 and other more recent NMOS CPUs.
https://www.eevblog.com/forum/projects/reverse-engineering-a...