The source of radiation surely makes a difference.
Directing the sensor at a small point source makes clustering higher
than if pointing it up into space [0] and receiving the "planar wave"
background radiation of the Universe.
I took a while to figure this out when measuring the audio clicks and
crackles from fire. I expect similar statistics to apply on a nuclear
level (physicists please correct me). Within small, local sources common
effects can be linked to common instigators. In other words events
beget events. So a local variation in some variable sets off a bunch
of related things [1].
As you sum this over an ever larger number of suitably decoupled
sources, the central limit theorem starts to apply and what was bad
uniform/even distribution becomes good Gaussian. In practice you need
more than the theoretical >12 sources, but once you approach a few
hundred uncorrelated sources the bell curve gets pretty good.
[0] probably assume the sky/space is an infinite number of sources all
at very large distances.
[1] In the (dangerous) limit imagine a near critical mass of Uranium
emitting bursts of chain cascades.