We have a comparison with Vault here: https://www.envkey.com/compare/hashicorp-vault/
We'll probably write up a comparison with Infisical soon as well but I'd say the main thing is that our end-to-end encryption has no opt-outs (as Infisical does for many of its integrations), and we use native apps and a CLI rather than offering a web UI. End-to-end encryption in a web browser offers minimal security benefit for reasons discussed in this thread: https://news.ycombinator.com/item?id=21838795 (the discussion is from 2019 and the original NCCGroup link from 2011 is now dead, but all the same issues still apply).
Also, I'm not sure if this has been addressed yet, but it has previously been noted that Infisical was completely lacking in automated tests. EnvKey has an extensive test suite ( core tests here: https://github.com/envkey/envkey/tree/main/public/app/tests and tests for all our sdks are included in each: https://github.com/envkey/envkey/tree/main/public/sdks).