Also, they do have some inherent beauty. I mean an aperiodic tiling is crazy right? And with one tile?
I was thinking more historically though. The development of those tools was driven by specific problems- classifying the behavior of higher dimensional spheres, determining if genus uniquely classifies spaces (not at all, but I believe people were once hopeful), even knot theory is an outgrowth of this kind of research.
Similar principle with Apple's laptop fan blades.
Same mechanism might be responsible for the Boson peak phenomena in amorphous materials and quasicrystals, where the macro-structure creates extra capacity for absorbing lower-than-lattice-frequency vibrations than what the crystal-structure alone predicts.
It's all about Fourier analysis.
One famous application of this is to encode these shapes using complementary snippets of DNA, to perform massively-parallel computation at the nano-scale: https://www.nature.com/articles/35035038
[1] https://commons.wikimedia.org/wiki/File:Rhombus_Penrose_tili...
2. Its important in technology and science (e.g quasi crystals).
3. They have an aesthetic some find pleasing.
Without a periodic crystal structure, it is likely to transmit light (see glass's transparency due to its amorphousness)
Being extremely hard and resistant they are used in applications like watch crystals, windows in grocery-store barcode scanners and armored car windows.