Generally, the most energetically favorable outcome is for these condensing molecules to incorporate into the 'ideal' location within the crystal lattice, forming a single-crystalline mass. From the images we can see condensation on walls of the container which indicates that 'non-ideal' incorporation is prevalent.
One way to combat this is to the raise the growth temperature, such that molecules that condense into non-single-crystalline locations are more likely to just dissolve back into the solution. Finding this optimal temperature where molecule-glass condensation is unlikely but molecule-crystal lattice is likely is, naturally, difficult.
Lots of nobs to turn in a process like this. It's fun to imagine how you might construct a proper growth reactor that allows more precise control of temperature and mass flux.