I was going to migrate over to ZeroSSL, but there were red flags in the form of missing documentation that you would expect from a CA, like what is the chain of trust for certificates that are being issued? If I have to issue myself a certificate to check which CA is being used to sign the cert, that doesn't feel right.
"Buypass Class 3 Root CA", which appears to be the root certificate they currently use, is present for all listed iOS versions (7+), which seems like a good sign. Let's Encrypt's "ISRG Root X1" is present in iOS 10+.
Similar lists for Android would be wonderful but probably impossible to compile due to ecosystem fragmentation. I guess there is no caniuse.com for root certificates.
ZeroSSL seems to have their chained "AAA Certificate Services" in the list for iOS 7 (until 2028)