The first thing I noticed is that this interface is discoverable - it shows me what I can do, which is incredible and makes me want to use it. The main reason I've been a casual tmux user and not an advanced one despite using it for years, is because every time I want to try something new I have to google if it's possible.
The second thing I noticed is that it uses ctrl-r as a core shortcut. Mega problem: ctrl-r is a built-in bash feature which I use every day to recall previous commands. This makes me think I can't use this tool at all.
I would suggest to consider taking a page from tmux's book. Just use a global modifier key. Ctrl-b is what tmux uses, so you know it's safe. Other software being developed knows they should avoid it, because tmux uses it. By also using it, you'd no longer have to dance around the global space of what shortcuts every software in existence is using. Additionally, if you use ctrl-b to enable your commands, you can minimize your interface. Currently you're using two entire lines to display your menu. That's going to become tiring as I use zellij 8 hours a day for years. I'll have to hide it eventually. Instead, what if you reduced it to zero lines? Put "ctrl-b: menu" in the upper right of your title bar. Pressing ctrl-b now enables commands and shows what your next keypress will do. You have now (1) avoided breaking existing shortcuts, (2) aligned with established standards (3) given some familiarity to welcome tmux users (4) expanded visible screen space and (5) simplified your menu system. You can also now remove ctrl-g since the interface is "locked" by default until I want to start interacting with it.
Anyway that's my 2 cents. Thanks for this exciting demo.