Lasers could cut lifespan of nuclear waste, a Nobel winner suggests
bigthink.com
bigthink.com
Transmuting elements with lasers is really cool for basic science, but completely useless as a solution for nuclear waste.
1: https://en.wikipedia.org/wiki/National_Ignition_Facility
2: https://en.wikipedia.org/wiki/Inertial_confinement_fusion
3: https://www.llnl.gov/news/nif-achieves-record-double-fusion-...
In the end it all boils down to the fact that visible light an laser operate on the energy scale of electronic transitions whereas nuclear transmutations occur at the vastly different energy scale of the strong force. This huge separation between electromagnetic interactions and strong nuclear interactions is btw also the reason why radioactive material is not typically green glowing goo.
You previous calculations are for creating light pressure sufficient for fusion, that's a uniquely energy consuming process, You can't reuse those numbers here because they are not trying to crush Uranium atoms together.
But likewise I could not find concrete details for the proposal.
The limit comes from the following process: Thanks to quantum mechanics there is an uncertainty principle between position and momentum. Less known it the uncertainty between time and energy. (If you have studied classical mechanic you will recognize that the variable pairs are the same that you know from Noethers theorem [3].)This implies that nature can (and will) violate conservation of energy by an amount deltaE for a time deltat up to hbar/deltaE. One such process is the creation of a electron-positron pair out of vacuum. That violates energy conservation by about 1 MeV and you have to return the (virtual) particles within hbar/1MeV or approximately 6e-22 seconds. If however the electric field is sufficiently large that the particles get accelerated to an energy of 1 MeV within that time they get to stay. An electric field that can do that has a field strength of 1.3e18 V/m.
At that intensity the laser light does not simply propagate through vaccuum as predicted by Maxwells equations, but is producing a pair plasma and gets damped. The process is fairly well described by QED. We are currently trying to get laser up to that intensity and to make accurate measurements of this QED effect as it does not only work for electron-positron pairs, but arbitrary particle-antiparticle pairs. Experimental deviations from the QED predictions would therefore imply the existence of additional light particles (and antiparticle) that we have not found through other methods.
1: https://en.wikipedia.org/wiki/Schwinger_limit
I'd bet that something lost in the translation or someone else would have pointed this out before.
And if you can read Russian, here a paper for your amusement for semisuccessful attempt to implement that: http://www1.jinr.ru/Pepan_letters/panl_2017_6/13_Andreeva.pd...
It contains a short English abstract which I copy here: The influence of laser irradiation on the gamma-activity of aqueous solutions of both 137Cs and 134Cs is experimentally studied in presence of Au nanoparticles at laser intensity of order of 10^(12)W/cm2. It is found that laser irradiation reduces the gamma-activity of both nuclides. This decrease is not accompanied by excessful gamma radiation in the spectral range of gamma-activity of their spontaneous decay. Possible mechanisms are discussed of the influence of laser radiation on the activity of isotopes on the basis of laser field enhancement on the plasmon resonance of nanoparticles.
(Aside: slow neutrons are often called "thermal" neutrons because they're in thermal equilibrium with the atoms around them. At room temperature they're going 2200 m/s, which corresponds to an energy of about 0.0253 electron-volts, slowed down from 2 million electron-volts when they emerged from fission)
A fast-neutron reactor ("fast reactor") is a reactor where the neutrons that emerge from a fission event are kept moving fast, simply by not putting a moderator into the design. These reactors use heavy nuclei or very low density material as coolants (sodium metal, lead-bismuth eutectic, helium, etc), so as to not slow down any neutrons. It takes much more fissile fuel to get a pile of nuclear fuel chain reacting in this configuration, but once you get it going, you get some very nice benefits.
Once started, fast neutron chain reactions have a vast surplus of neutrons going around. This is for two main reasons: (1) The number of neutrons emitted per fission increases dramatically as the neutron speed increases above a threshold around 1 MeV, and (2) parasitic absorption of fast neutrons is low for all nuclides. With so many extra neutrons around, you can afford to put extra "stuff" in your reactor, such as spent nuclear fuel (nuclear waste) or extra fertile material (uranium-238 or thorium-232).
You can make these reactors into breeder reactors (which convert U-238 or Th-232 into fissile fuel in such a way that could power the entire of humanity 10x over for a few million years, at least, using known resources), or you can make these reactors into burner reactors, whose job it is to transmute used fuel from other reactors into shorter-lived material (similar to what OP's article is about, but much more practical).
A definitive guide to understanding transmutation of spent fuel in fast-neutron reactors is put out by the UN's International Atomic Energy Commission [TRS-435]:
"Implications of Partitioning and Transmutation in Radioactive Waste Management" https://www-pub.iaea.org/MTCD/Publications/PDF/TRS435_web.pd...
A handful of fast-neutron reactors have been built, starting with tiny single critical mass assemblies in the 1940s, to the first true demo of breeding more fuel than you consume in EBR-1 in 1951 to the EBR-2's safety demo weeks before Chernobyl showing that the reactor could passively shut down and cool itself without any human intervention or external power or control rods inserting, to India's PFBR fast reactor that's been under construction for the past 18 years.
Only the Russians have successfully operated fast reactors commercially, via the BN-350 and BN-600. In general, fast neutron reactors are considered more complex and expensive to build and operate than traditional water-cooled thermal neutron reactors.
We once thought uranium was very scarce, and so we put a lot of money into fast breeder reactors. Then it turned out that there's lots of uranium and fast reactors are largely on hold internationally. France just announced the cancellation of its national fast reactor program (ASTRID). Russia delayed their next BN fast reactor, saying their VVER (slow neutron) reactors are bout 4x cheaper. China and India are pushing forward. The US shut down its last fast reactors (EBR-II and FFTF) in the early 1990s. Many nuclear startup companies are now exploring options to get back into fast reactors.
The US DOE is putting forth a major project to build a new fast reactor very similar to the FFTF, but in Idaho instead of Washington and with metal fuel rods instead of oxide ceramic ones. The project is called the Versatile Test Reactor (VTR) and is actively discussed in current nuclear news.
Fast reactor tech hasn't been popular because it's more expensive than regular old water-cooled fission reactor tech. To keep neutrons going fast you have to use exotic coolants like sodium metal. Since you don't want to mix a chemical hazard with a radiological one, you insert an additional intermediate heat transfer loop into the system. Hot radioactive sodium transfers heat to hot non-radioactive sodium which transfers heat to water which boils and turns a turbine to crank a generator to push electrons around to provide low-carbon service to human quality of life.
Molten sodium is easy to pump, non-corrosive to many metals including steel, and a good heat transfer medium. The chemical industry uses it routinely. In a nuclear reactor, it would also chemically sequester a particularly annoying fission product (I-131) in case of a fuel element leaking. Unpressurized, it is good up to 800C before it boils.
By contrast, water at 300C will corrode most steels. At higher temperature, it will corrode zircalloy, forming hydrogen. And it really wants to be a gas, hence the giant containment buildings around LWR.
What did you say? "But sodium explodes in contact with water?" That's easy to solve, just keep the water out. A sodium cooled reactor should be coupled to a supercritical CO2 turbine instead of a steam turbine. That removes the problem of leaking and exploding heat exchangers.
(Footnote: I like molten salts better than sodium. But sodium is still better that water.)
Have you ever studied a detailed procedure for heating up a large sodium valve from the solid sodium phase to the liquid? If not I highly recommend doing so. It's truly remarkable. Molten salt systems are the same level of complexity, but much more radioactive in the primary system. Remote maintenance of this stuff is totally doable, but it sure as hell is exotic. Rickover's characterization of sodium systems stands to this day.
Traditional sodium systems with void-swelling resistant structural materials may not go to high enough temperatures to strongly justify the tech development needed for a sCO2 balance of plant in the short term. Sodium-water steam generators with leak detection have worked well-enough to build a few more of them while sCO2 turbomachinery gets figured out at the 100s of MW scale.
Becoming a nuclear superpower weeks after operation of a fast-neutron reactor is a bit of an overstatement.
Fast reactors enables breeding, that is producing more fissile material from the fuel than is consumed. They are also better at burning up various isotopes that thermal reactors have trouble with.
We have many dangerous devices extremely close to the population already. Cars kill more people in a year than all nuclear reactors have killed in the whole time of their existence. Should we bury the cars underground instead?
No, not Chernobyl. I'm talking about EBR-II, a fast reactor. Nothing happened. That's how dangerous the device is!
On the other hand, water at 300C and 200bar will explode spontaneously without coming into contact with anything. A steam explosion is no fun, according to Wikipedia.
https://www.forbes.com/sites/realspin/2014/10/01/why-doesnt-...
"erraPower notes that the US hosts 700,000 metric tons of depleted uranium and that 8 metric tons could power 2.5 million homes for a year.[9] Some reports claim that the high fuel efficiency of TWRs, combined with the ability to use uranium recovered from river or sea water, means enough fuel is available to generate electricity for 10 billion people at US per capita consumption levels for million-year time-scales."
That sounds completely crazy haha
Do you know how rare, useful and valuable those heavy atoms are?
The tunability of this gamma rays source makes it possible to target and induce nuclear reactions in unstable atoms.
If I remember correctly, when I saw the seminar talk by the originator of the concept, a few years ago, he said that an existing super-conductor-based linear accelerator in Japan could feasibily by modified to generate enough gamma rays to burn thousands of tons of radioactive waste per year. (Don't quote me on the exact amounts, though, it's been a while).
Are they talking about transmutation with lasers? Would it work for Lead -> Gold too?
That's just a cube 28m on a side, maybe the same size as a small apartment block.
Just dump it into a subduction zone
With such a small volume I think 'do nothing' is fine at the moment until we can find an economical use for it (fast breeder, traveling-wave etc, etc), or agree the best way to dispose of it - 20,000-year managed repositories don't seem viable to me.
The actual proposal isn't to irradiate nuclear waste with lasers. The idea is to use the laser to accelerate protons, irradiate heavy nuclei with those protons to get them to either fission or at least emit neutrons, irradiate long-lived waste with those neutrons to transmute it. It's possible in theory.
In practice, it's nonsense. These accelerators have low efficiency and produce few neutrons. This makes the process slow and inefficient. So inefficient in fact, that all practical (for small values of "practical") proposals are actually for sub-critical reactors that use nuclear fission to amplify the neutron output.
But then the idiocy becomes clear: instead of a sub-critical reactor and an unbelievably expensive accelerator, you might as well build a critical reactor, recycle the actinides directly and maybe transmute the fission products.
In other words, this is a guy who just likes particle accelerators. He has a solution, now he's looking for a suitable problem.
Short of neutron guns, are there environmental conditions that affect nuclear half-life?
There is much to be learned in this space still.
Wouldn't this basically boost mpg and/or increase safety of reactors?
One problem would be transporting it, but again, solvable problems, we tanker oil around the world, so it can be done. The trouble is though political. No one wants all that nuclear waste in their back yard, even if no one ever uses the backyard.
Fukishima added to the problem - if the Japanese, whose engineering skill is the best in the world, have problems then what about the rest of the world? I see this as a very valid objection.
One of the problems I see in the popular mind is the idea that radiation is somehow unique and only occurs in nuclear reactors, and any of it appears somewhere then we're all dead. The coal industry makes sure no one finds out that the amount of radiation expelled by coal powered stations exceeds that produced by nuclear reactors https://www.scientificamerican.com/article/coal-ash-is-more-...
As you say the amount to be stored is pretty small, and could probably be dumped down a hole in an afternoon and home in time for tea
An anecdote - I went to a radiology clinic a while ago for a tour (writing some software) and we stopped by the room where they store the radioactive material, pretty low level stuff and all stored away. The manager taking me around said "This is where we store the radiocative stuff" looking at me and waiting for a reaction - a bit of fun I imagine he has - expecting me to run away and panic, but I have a physics degree so no drama - he was disappointed, and we laughed. But this is the public mind - radiation is scary stuff that causes mutations and kills you, so there's a real marketing problem. No doubt this has been pumped up by the oil and coal industry over the years.
The only scenarios that people have presented in which nuclear waste could result in contamination are borderline absurd, like if humanity hypothetically loses all records of where waste is buried along with knowledge of what radiation is and some future civilization might dig up the waste canisters and crack them open.
However, anti-nuclear activists deliberately focus too much on the problem of storing it indefinitely in the near term.
If we plan storage for tens of thousands of years, waiting out a few hundred years for economic and technological development is in order. The waste of tomorrow might be the fuel of the future.
How did you arrive at that number? The waste is harmful for hundreds of thousands or even millions of years.
Like I said, I think the "indefinite storage" question is a red herring posed by anti-nuclear activism.
Perhaps a better question would be: How much we should be concerned about the inhabitants of this planet in 10,000 years when supposedly there's a mass extinction coming up in the next 100 years due to the energy needs of today and yesterday.
The reality is, nuclear waste should mostly be treated similarly to the toxic waste that is generates by other sectors of heavy industry.
https://space.stackexchange.com/questions/13396/do-any-curre...
Sure, you would encase them in something that could survive reentry or detonation of the rocket. Choosing a launch location and trajectory for easy recovery is also possible.
However, paying 1,000+$/lb to get rid of Nuclear waste is extremely expensive. Simply storing it in a pond for ~120 years and the stuff gets vastly less radioactive as short half-life material decays. Strontium-90 and cesium-137 have half-lives of about 30 years so you get 6% as much of them and essentially everything with a shorter half life is gone. Plutonium-238 has a longer half life of 87 years, but you also get rid of ~2/3 of that.
You still have almost off the Plutonium-239 with a half-life of 24,000 years, but that stuff is not nearly as nasty and can be reprocessed for fuel. Further, reprocessing becomes cheaper after waiting for it to cool down.
PS: Plutonium-238, Strontium-90 and cesium-137 can also be used for space probes via: https://en.m.wikipedia.org/wiki/Radioisotope_thermoelectric_...
For now, the solution is to use nuclear fuel in the most efficient manner so as to minimize waste.