He made other incorrect predictions in the same document. We continue to (incidentally and carelessly) change the climate, but have yet to achieve anything like the reliably controllable weather he anticipated.
He also incorrectly anticipated that atomic transmutation of the elements would become a bigger trend than chemical rearrangement of existing elements.
"It is worth emphasizing that the main trend will be systematic exploration of nuclear reactions — that is, the transmutation of elements, or alchemy rather than chemistry."
As for why he was mistaken about nuclear power, it's possible that he was extrapolating from the fantastically rapid progress of nuclear weapons technology. Fission was demonstrated in 1938, the first chain reaction in 1942, the first fission weapon in 1945. The first megaton scale thermonuclear explosion was demonstrated in 1952 and serial production of thermonuclear weapons began in 1954. Between 1944 and 1954 the explosive power of the largest military bombs went up by a factor of roughly two million [1] [2]. There was a 2300-fold leap from Grand Slam to Little Boy (6.5 tons TNT equivalent to 15 kilotons) and another thousand-fold leap from Little Boy to Castle Bravo (15 kilotons to 15 megatons).
The challenges of making useful power reactors for electricity production are much different. Civilian power reactors have to compete with other electricity sources on cost. They have to produce power for decades rather than a fraction of a second. They are expected to fully contain fission products rather than disperse them widely as fallout. Recall that at the time of this writing, 1955, no country had yet built a power reactor comparable in output to large coal or hydroelectric plants. There had only been some small demonstrations like the 2 megawatts of electricity produced by the BORAX-III reactor. The actual difficulties to be encountered at larger scales were not yet known.
Finally, "affordable" electricity was a moving target. In constant dollars, large American industrial buyers were paying 40% less per megawatt hour in 1970 than they were in 1950 [3]. Concerns about acutely hazardous air pollution were not yet widespread enough to justify a cost premium over fossil-generated power. Widespread concerns about greenhouse gas emissions were even further off.
[1] https://en.wikipedia.org/wiki/Grand_Slam_(bomb)
[2] https://en.wikipedia.org/wiki/Mark_17_nuclear_bomb
[3] https://www.census.gov/history/pdf/histstats-colonial-1970.p... - page 827