The film has the better supporting cast by far[0], but the original series is worth watching just for that portrayal. Watch his face as he slowly puts on his glasses during the beginning of the interrogation scene with Ricki Tarr for example.
[0] with the possible exception of another great performance by Ian Richardson
Edit: I very much enjoyed the film too, including Gary Oldman. But the miniseries captured the bleakness of the era, had time to explore more of the detail, and left more things implicit rather than explicit. All styles of production that I personally enjoy.
The old TV series had a superb ensemble cast. The new one in some ways let itself down. Hungary for Czechoslovakia. Turkey for Hong Kong. Peter Guillaim has a gay lover. Minor changes but also.. why?
For example (warning: potential spoilers, though you'd have to be pretty super attentive to detail if you ended up noticing this the first time through the film):
https://movies.stackexchange.com/questions/91858
Fortunately, it is (or was) on Netflix so I was able to do that.
I probably watched it at least a dozen times and with every viewing I would still manage to find some new little meaningful detail I had missed before. If I can't find anything new that interests me on Netflix (not hard), I'll usually just queue it up again. Great film.