"secure" probably refers to the sandboxing functionality that Chrome has had since version 1.
This proprietary software apparently allowed for sending Google every URL a Chrome user types in (http://www.favbrowser.com/google-chrome-spyware-confirmed/) and making it easy for extensions to spy on Chrome users (https://labs.detectify.com/2015/07/28/how-i-disabled-your-ch...) which many Chrome extensions apparently do, or activating a Chrome user's microphone and sending the captured data to Google (https://www.privateinternetaccess.com/blog/2015/06/google-ch...). Hardly behavior users are likely to call "secure" because such behavior does not look out for the security of its users, but instead securing access to Chrome user's data.