One person can hold 1 or 5000 addresses, it doesn't make sense to draw pretty plots from it.
So, while I appreciate the great effort to quantify the level of decentralization in the cryptocurrency space, I think the article mostly just exposes the subjective decisions being made by people who make claims about decentralization. Even that could be a big step forward for debating these technologies, though.
It seems the article is mostly to reframe the discussion.
I haven't even seen bad versions of these measures compiled before. Debating the choice of bucketing strategy (and other such) is a massive improvement.