There aren't enough pins. Certainly not enough pins accesible in single-cycle reads/writes. Maybe you could multiplex them with external hardware to talk to a SIMM but you'd be talking to memory at single megahertz effectively.

An SDRAM controller in an FPGA on the other side of the QSPI link would be faster, but it'd still be slow. You could get it to work to say you've done it, but it'd run at literal-days-to-boot speeds.

The board (and chip) is meant and marketed for freetards who like Arduinos - so I bought one and so did several of my friends. LEDs were blinked and better futures dreamt of. It's cool. But it's not a workstation chip by any stretch of the imagination.

Hopefully the next version will have a real external memory bus.