I would say the main deficiency with MARTA's buses is frequency, not the number of options. MUNI's buses run way more frequently I've found when visiting SF.
Sidebar: I currently live in Portland, which has an award-winning bus/rail service. And it is true, it's awesome. The drivers are polite, and often really care about urban planning/civic stuff. The buses are clean, the documentation/data/maps/API well-done.
But because Portland is so much less dense than SF, it still means that in many cases, taking a bus here is more of a drag, and cars more common. (On a personal note, I've gotten way more into biking since moving here from SF.)