Turning CO2 to Stone
sciencebulletin.org
sciencebulletin.org
Total worldwide carbon production is 38.2 billion tons per year. Cost to sequester a ton of carbon is between $30 and $150, depending on who you ask and how you do it. Let's assume a middle of the road price of $90/ton. That's $3.438 trillion a year, or about $478 per person. This is roughly equal to the US yearly federal spending, or 3% of the world GDP.
If you somehow pooled together all the world's billionaires and got them to contribute their annual income (roughly $600 billion a year, averaging the past 7 years) to the effort, you could eliminate roughly 20% of carbon produced in the world every year.
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Suddenly, it becomes crystal clear why finding new sequestration methods is incredibly important: if you can get the cost from $160 to $10 per ton, then suddenly all you'd need would be a coalition of half the world's billionaires to stop the main cause of global warming.
Additionally, it's important that people realize that CO2 production is in tons of CO2 per year. Tree offsets are a one-time deal, since when trees die they release CO2, and when new ones are born they absorb that CO2 again. After they've been planted, forests are generally carbon neutral. That's why we can't "just plant trees": we'd have to be continuously planting new trees. The Earth is only 8% arable land, much of which already has stuff on it, or is undesirable for one reason or another. We'd run out of space pretty fast. Trees are good for other reasons: preventing climate change (different from global warming), preserving species diversity, being nice to look at, etc etc.
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Mostly off-topic: when I was looking at estimates of land size, apparently the amount the US has shrunk from 2007 to 2015 (14,000 km2; went from 9,161,120 km2 to 9,147,420 km2) [0] is roughly equivalent to half the area of the Netherlands. Wow.
OTOH, the total cost (not just for sequestration) is about $100, maybe a bit more, in most estimates.
For reference, a gallon of gas produces 20 pounds of CO2, so $100/ton equals $1/gallon of gasoline. That's roughly what you'd have to increase gasoline price by to fund CO2 capture, transport and storage. (This neglects that the capture part is neigh-on impossible.)
For electricity, to compensate for the average US CO2 emissions per kWh (~1.2 lbs/kWh), you'd have to increase the price by about 6 cents per kWh.
To do CCS for both gasoline and electricity consumption, the average US family would have to pay (order of magnitude) 1000 x $1 + 12000 x $0.06 = $1720. That would compensate for about half the family's CO2 emissions. The remaining half is dominated by emissions from the food we eat, the stuff we buy and from having fun.
is that really true? If a tree died, i would assume the carbon is either buried, or otherwise remain solid, unless it's burnt.
By default about half of a tree's absorbed carbon is injected into the ground to build soil, as root mass and root exudates. Plus trees drop mulch -- mainly leaves. Soil carbon is only released when the soil is destroyed or eroded away. So... don't do that. :)
"Based on a genetic analysis of mushroom fungi, it was proposed that large quantities of wood were buried during [the Carboniferous] period because animals and decomposing bacteria had not yet evolved enzymes that could effectively digest the resistant phenolic lignin polymers and waxy suberin polymers. They suggest that fungi that could break those substances down effectively only became dominant towards the end of the period, making subsequent coal formation much rarer."
https://en.m.wikipedia.org/wiki/Carboniferous See Rocks and Coal
Moral of the story: you should start regular forest/grass fires to turn the stored carbon into charcoal. A biologist can give you a number of other reasons why this is good for the forest as well: common knowledge about forest fires is almost completely false.
The implication being that we have one good shot at solving civilisation. It just gets more difficult when we start to run out of fossil fuels.
One of the reasons we don't see anything going on out there when we look up could very well be that most civilisations never properly make it off their planets.
Can anyone else comment on this that might have better information than me?
The global potential of energy from hydroelectricity is only a small fraction of our current fossil-based consumption, though. And while wind and solar have potential resources far past fossil power, they can't expand as fast as fossils did historically. So the Fermi Paradox aspect might be that civilizations without fossils and without the self-control to limit reproduction are hobbled by cycles of Malthusian collapse. Or perhaps space-capable civilizations that didn't fall into the Malthusian boom-bust trap while still confined to one planet also don't go crazy with growth once they escape their gravity well, so they're out there but not leaving evidence dramatic enough to be seen by our current telescopes.
http://www.hitachiconstruction.com/about/media-press-release...
http://www.oemoffhighway.com/article/11224086/electrificatio...
If you just mean that it's impractical to build the electrical grid out to a remote mining site, that's true. In the present day remote mining sites typically use diesel fueled generators, now being supplemented with photovoltaic arrays in sunny regions. If you imagine a world with approximately-1940-level technology (so PV is not yet an option) and no fossil fuel, then you'd need to use something like biodiesel or ethanol instead of fossil-derived diesel.
Yes, that was the general issue. We do a lot of mining in remote sites that don't have hydro power or any realistic way to get it there. You could use biofuels, but it's hard to imagine bootstrapping a technical society to the point that that becomes feasible without prior use of fossil fuels.
[1] http://www.lowtechmagazine.com/2013/01/mechanical-transmissi...
Well, we are busy recycling that one. All that carbon in the atmosphere will likely eventually precipitate out. On a geological timescale oil is renewable; it's simply that humans don't live that long. I suppose the cockroach civilization 60 megayears hence will be able to power their vehicles that way.
Or, you could be one of the few who believes the abiotic theory of oil production. I'm not one of them!
You misunderstand the purpose of trees. They're basically solar powered, organic carbon sequestration devices that happen to run for free. If we ever run out of space to plant trees, we can just cut some down, reduce it down to charcoal and bury it back into the ground which conveniently leaves a readily accessible fossil fuel source for our ancestors in the case of civilizational collapse.
But we're still a long way away from running out of room to plant trees. We're still desperately trying to plant enough trees to stop the encroaching of the Sahara and there's vague, futuristic plans to try and turn the entire Sahara into a forest. Similarly, China is desperately planting trees to stop the encroachment of the Gobi.
If you're removing carbon from the air by burying trees then you'll only be able to sustain the energy intensity of civilization in the Britain of 1800, plus what we can get with renewables. What this new form of capture gives us is the ability to get rid of excess carbon without using huge amounts of arable land to do it.
There are plenty of high-power ways to make energy without carbon. The question is if enough of the population can accept it.
Yes, that's the point. Plant trees, cut them down when mature and plant new ones. Use the harvested trees to make cross laminated timber and other engineered wood products and use these to replace concrete and steel (which also release CO2 during production). As long as the timber doesn't burn or rot the carbon is stored permanently.
Why not just let nature do it's job? If too much CO2 will kill us, then it's a self regulating system. It happened before with the Azolla event. You get fewer humans, more plants, everything else gets a chance to die off or recover, maybe a new species takes over.
Why bother with carbon sequestration?
Jesus, grow some empathy.
Rather than store carbon in solid form, which in fact plants (rainforest and such) already do anyway without the unecessary expense, why not close coal fired power stations and build nuclear? They're safer and the waste is negligible compared to coal and can be further reduced (breeder reactors, thorium cycle etc.). Burning coal also throws heavy metals (Mercury and Arsenic to name a few) and SO2/SO3 into the air. Carbon dioxide is the least of coal's problems because it can be fixed by plants or turn into bricks with additional expense.
They will just release their carbon content back when they are burned or transformed in any other way that only the mineral content is left. Otherwise, paper still contains carbon. Coal (buried, not burned) contains carbon. Furniture, houses, anything you make with wood will be a way of storing carbon.
You just also need to supply water and solar light. They will grow. Simple and efficient.
Crucially, the activation energy for the weathering of silicates to carbonates is low in the presence of water and carbon dioxide. Low enough that it happens spontaneously in nature on exposed rock surfaces. That means that the energy inputs required to reduce atmospheric CO2 via silicate weathering are much lower than a "combustion in reverse" process to turn gaseous CO2 into synthetic coal and bury it.
The other crucial issue is that the kinetics of silicate weathering are tremendously hindered in nature. A freshly fractured basalt surface weathers rapidly for a year or two and then develops a cation-depleted micron scale "rind" that drastically slows the weathering reactions with the rest of the bulk rock.
One way to accelerate the kinetics of silicate weathering is to use more concentrated materials, like the Iceland injection process: nearly pure CO2 plus water will react much faster than natural surface waters exposed to hundreds-of-ppm CO2 in the atmosphere. That works ok if you have a rich stream of CO2 like directly from a power plant's stacks. It won't work for dealing with CO2 already emitted to the atmosphere unless you add a complicated and energetically expensive pre-concentration stage to turn 400 ppm of atmospheric CO2 into a 950,000 ppm CO2 stream you can inject.
The other way to improve the kinetics of silicate weathering is to generate a lot more surface area: crush bulk stone into particles 100 microns or finer. Then there's a lot of fast-reacting extra surface area that can react with CO2 at ambient concentrations. And even the slow weathering to the center of the particle will take maybe a century rather than multiple millennia. (If a century sounds unacceptably slow, I would venture that you have not fully internalized the vast timescales that unaided nature would take to restore the pre-industrial CO2 equilibrium.)
Putting crushed stone particles in near-shore ocean environments may further accelerate weathering by ensuring that natural wave action keeps abrading the rind from particles. Crushed stone rich in magnesium and calcium silicates can also be applied to acid sulfate soils in tropical agriculture. Raising the pH of acid soils increases agricultural productivity by preventing low-pH aluminum toxicity to plants and, unlike sweetening soil with limestone, it sequesters some carbon at the same time. The crushed stone accelerated weathering approach can offset all sorts of CO2 emissions: point or distributed sources, local or distant sources, present or past sources. Finally, it restores the historical pH balance of the oceans as well as getting rid of excess radiative forcing from CO2.
The amounts of stone required to offset historical emissions are vast, but any solution will be vast because the scale of the problem itself is vast. In terms of scalability, simplicity, energetics, and flexibility, I think that accelerated silicate weathering is the best shot at long term restoration of oceanic and atmospheric CO2 concentrations to the pre-industrial baseline.
Or does it mean that the time of planting trees and preserving forests is over now and we have to do it another (most often less efficient) way?
Under what conditions does this happen?
I have no idea if this stores any carbon anymore though.
Nonetheless, plants have important benefits, since they alter the local climate by changing the albedo and perspirating. Perspiration of plants in jungles helps to create clouds and regulate humidity, and would help to counteract some of the negative effects of climate change.
Playing devil's advocate here, water vapor is an incredibly powerful greenhouse gas, even more so than CO2.
They refill coal mines, plant trees where there were once cities, and silence radio emissions so that everything appears to be in its "natural" state.
We seem to have forgotten that natural forests are incredibly productive, and don't need artificial fertilizer. So we have a proof-of-concept. How do they do it, and how can we emulate those processes?
Spoiler alert: soil (along with the root action of plants) is essentially a flat biological nanomachine that breaks down solid rock and fixes nitrogen, manufacturing fertilizer in-situ. https://www.youtube.com/watch?v=x2H60ritjag
Of course the logical way to do this is not to create some vast new land use category ("carbon forests" or similar), but to transition our largest current land use category -- agriculture -- from a carbon-releasing to a carbon-sequestering mode. It also helps to increase biomass per hectare in suburbs, by transitioning our current low-carbon-density lawns over to a biome that buffers substantial amounts of carbon.
This is the fundamental insight behind Permaculture btw, which has been working on figuring out exactly what this looks like. It's a hard problem yes, but one with existential importance for humanity.
>Biochar is basically coal, which could be burned and converted into CO2 again.
...so don't do that. :) It's it obvious that burning coal also needs to stop for effective climate mitigation?
In this application, density matters. Biochar is extremely low density, and high in surface area, which makes it an ideal soil amendment which buffers rainwater and provides microbial habitat (not to mention raw carbon for building into soil biomass). By contrast actual coal is nearly worthless in this application.
Most the CO2 from fossil fuels comes from ancient bogs, where plants were prevented from decomposing for long enough that they could eventually turn into materials like coal and petroleum. In essence, they were a result of taking plant matter _out_ of the biosphere, which is sort of the opposite of hugelkultur's goal.
In that context, you will have a net-positive CO2 absorption (or, a net-negative CO2 release into the atmosphere).
Or you can sink it in the Baltic, where nothing consumes it.
Is it? Let's do the math.
Absorbing the 350 teratonnes of human emitted carbon[1] over the 8.4 billion hectares of Earth's non-tundra / non-desert land surface area[2] works out to... 42 tonnes per hectare. If we can green deserts[3] that drops to 30 tonnes.
That's 30-40 trees per hectare, at 1 tonne per tree.[4] Or 3 kg per square meter of soil carbon, the equivalent of 25-35 cm of topsoil. More likely some combination of the two. Soil carbon is stored up to 40 meters down by deep rooted plants.[5]
Most of our land management is via agriculture, so agriculture seems to be the only lever long enough to make a dent. Practically this implies transitioning from soil destroying tillage to soil building cover crops, long-distance imported fertilizer to in-situ fertility produced by soil organisms, and ecologically unstable monocultures to resiliant polyculture, agroforestry, and rotational grazing systems.
The "gotcha" question is not whether we can replace our existing agriculture with these systems. The question is whether we can replace our existing agriculture with itself. Any unsustainable system is, by definition, not a viable replacement for itself.
[1] http://petrolog.typepad.com/climate_change/2010/01/cumulativ....
[2] http://cnx.org/contents/TWFXbERo@1/The-main-biomes
[3] https://www.youtube.com/watch?v=2xcZS7arcgk
[4] http://cabiblog.typepad.com/hand_picked/2011/06/ever-wondere....
Unfortunately "long-distance imported fertilizer to in-situ fertility produced by soil organisms" cannot work if food is exported off of the farm. Every gram of food taken off the farm includes some micro-nutrients - various minerals that are required for life that have been removed from the soil and taken elsewhere.
>Unfortunately "long-distance imported fertilizer to in-situ fertility produced by soil organisms" cannot work if food is exported off of the farm.
It's not like there's a shortage of rocks (where soil bacteria and deep rooted plants harvest and dissolve micronutrients) or air (the source of carbon, as well as nitrogen fixed by rhizobium bacteria in root nodules). Soil tests only look at dissolved nutrients, not those yet to be released from the minerals in rock, which range in size from bedrock to clay. This is detailed in the video I linked.
But it certainly helps if you recycle human waste into fertilizer, rather than just releasing those nutrients into waterways (and ultimately, the ocean) or landfills. The key is to close the fertility loop while also interrupting the fecal-oral route. Thermophilic composting or biogas digesters can do this on a small scale, and systems like those used by Milorganite can do this on a city scale.
It's more meaningful to reason about co2 storage in terms of area dedicated to plants, than the plants themselves.
That's not true, a stable mature forest is a long-term carbon store, the release from decomposition being offset by capture by new growth.
And depending on the underlying soils it may be a net sink until it's clear cut and burned away (e.g. peat swamps as in south-east asian islands).
Growing forests are carbon sinks, until the forest stops growing (and it becomes a carbon store)...
http://www.wri.org/blog/2013/11/carbon-dioxide-emissions-fos...
Total carbon stored worldwide in biomass, dead wood, and soil is about 640 Gt.
ftp://ftp.fao.org/docrep/fao/010/i0105e/i0105e04.pdf
Of the 550 Gt of carbon humans induced into the atmosphere since 1870, 390 Gt was emitted directly (through burning, cement production, etc), and only 160 Gt was through deforestation and other land use change.
That's a nonsensical argument and quite literally missing the forest for the tree.
[1] http://www.ipcc.ie/a-to-z-peatlands/peatland-action-plan/cli...
Ok, but let's be careful not to exclude the middle here. "We got here by mining (an industrial activity), therefore we can't use plants in any part of a carbon sequestration chain (even one that also involves industrial activity)." Trying to use this argument as a blanket ban on plants becomes little more than an appeal to sympathetic magic.
The only thing that matters is how much CO2 a technique can buffer (annual production x time constant), not whether or not it uses plants at any stage. Plants already have enormous annual production, but for economic/thermodynamic reasons it's hard for purely factory-based techniques to achieve sufficient scale. It becomes a money sink both up-front and operationally, respectively because A) factories are expensive, and B) hard thermodynamic constraints mean that it's at a fundamental competitive disadvantage compared to any typical [reminder: energy consuming] factory.
Not sure where your logic is coming from here. I am not saying we shouldn't use plants, but I am saying that even if we let forests retake "all the land," the stable CO2 level would be a bit higher than pre-industrialization, and it would stay that way for a long time until dead plant matter returned significant amounts of carbon to the deeper parts of the crust.
Therefore, using other methods like the one in the article are necessary if we want to reduce CO2 levels.
I agree, a hands-off approach is insufficient. We would need to actively manage those forests (which is just as unnatural an activity btw), using intelligent design to improve upon the carbon density possible solely from blind natural processes.
Big industrial thermodynamic sinks don't scale (and imo never will), simply because they can't economically compete with conventional energy consuming factories. An approach is needed that sequesters carbon while also producing sufficiently valuable goods to society (ie probably not rocks). Food is one possibility, and can avoid carbon futility since in perennial systems the annual food yield is a small percentage of the total carbon stored in the biome.
Carbonates are among the most common minerals on earth, particularly as calcium carbonate in its many forms. Calcium carbonate is slightly soluble in water and subject to degradation in acidic environments. While hardly an impervious carbon dioxide store, that's a benefit in that its easy degradation makes it an extremely useful mineral supporting essential infrastructure industries.
IOW sequestering carbon as carbonates doesn't imply the CO2 is inaccessible but simply not reduced to an elemental or hydrocarbon form readily usable as an energy source. It's a trade-off between storage in an easier/quicker non-energy form or a protracted/difficult-to-implement energy-source form. Worth considering that in geological time the carbonate vs. carbon storage pools will probably "even out" since both are clearly mutable.
And you can't just plant forests everywhere, for example china experiences issues with its Green Wall, where the trees soak up so much water that it causes the ground water level to fall.
Below is the original comment with correction for accounting error.
_________
$15 per person per US person[2] per year does not sound like a lot, but in sum per year it's a massive amount of money; amount would be $4,847,228,805.
For example, per person using the 2014 net collections[1] of the US's net tax collections divided by the population estimate for July 2016[2], the US revenue per person is $8,000.
[1] ($2,690,755,432) https://www.irs.gov/uac/soi-tax-stats-collections-and-refund...
[2] (323,148,587) http://www.census.gov/popclock/
On the spreadsheet, money amounts are in thousands of dollars.
At the point you're spending billions in sum in a country for a reoccurring & necessary theoricially non-profit service, it would make more sense to do this via the government; yes, I get it's not a requirement, assumes government is functions efficiently, etc.
https://news.ycombinator.com/item?id=13457660
Thanks for posting an update - if the titles not right, just post a comment and I'll update it.
Some of the carbon offset organizations that plant trees are having a hard time finding people and land to do the work, since cash crop trees tend not to be good carbon collector/stores, poor farmers tend to forego the pay-for-trees to be able to grow cash crops.
I don't know the specific organizations, but I have heard that this can be a complication issue.
https://carbonfund.org/projects/
It'd be great if any of these had published progress reports (not to say they don't but I haven't read them). Seems like you could fake one of these pretty easily if you tried.
If you want to reverse the process you need some energy, so what would be the point of burning the oil in the first place?
Or you could envision large carbon sequestration plants powered by on-site nuclear.
I'm not sure I understand, you're suuggesting that we
1. Burn oil to produce energy (and CO2 as a byproduct)
2. Use the energy to do X
3. Use non-fossil energy to get rid of the CO2 we created during step 1.
When we could just do:
1. Use non-fossil energy to do X
Am I missing something?
Fossil fuels are incredibly energy-dense and convenient to transport and work with, while renewables aren't. There's plenty of transport systems that are utterly reliant on fossil fuels and couldn't be converted to renewable energy. Carbon sequestering would allow continued use of these while staying carbon-neutral.
We shall see. For whatever it's worth, Tesla's CEO disagrees. https://www.youtube.com/watch?v=0871VJfvD1c&t=57s
>I think all transport, with the exception of rockets, will go fully electric.
This is the most recent example, but he's been saying this since at least 2013. Surprisingly, he's also made it clear that he thinks this applies to ships and planes too. http://www.digitaltrends.com/cool-tech/elon-musk-electric-ai...
Ships probably will see batteries as an asset: they can place them in ideal locations for weight distribution/stability.
You certainly can't get there by taking an existing aircraft, removing the fuel and replacing it with batteries. It's the same fallacy as the gasoline automakers make with electric cars, and it results in a worse vehicle design. The whole system has to be re-imagined from the ground up to exploit the advantages of electric propulsion.
Several of the design concepts for his proposed supersonic VTOL electric transcontinental commercial jet airplane have already been revealed:
* The plane would fly at high altitude, somewhere around 80,000 ft. Combustion airplanes have a 30-40,000 ft ceiling limited by the need to ingest oxygen. Due to the exponential decay of density with height this dramatically reduces drag, thereby reducing engine power and structural stress. Coincidentally this is also higher than almost all bad weather.
* VTOL is easier since electric motors have a better power:weight ratio than turbine engines. This eliminates constraints due to runway length and width, and means the wing can be more closely optimized for cruising. It also means smaller airports are possible, reducing gate fees.
* The wings also don't need to double as liquid fuel tanks, and don't need to handle different stresses when empty vs full.
* A high mass fraction of batteries compared to combustion aircraft (mid to high 70% range). Energy density at least 400 Wh/kg (which as you point out, is still much lower than kerosene).
* Eliminating the tail section in favor of gimbaling the electric fan, again reducing drag and weight.
* You also get about a 1% drop in weight compared to existing jets due to reduced gravity and centrifugal force.
A good video compilation of quotes is https://www.youtube.com/watch?v=erjdYiwoYAo
Of course mountains are often a factor. There are deserts at the base of forested mountains. The mountain takes all the rain.
Also related: oil, peat.
It would be easier to replace as much coal as possible with other forms of energy as soon as possible.
We just had an article on HN where Wyoming banned renewables.
I can't wait to see nuclear power plants selling oil and gasoline.
(Gasoline on US bases in Afghanistan ended up costing something more than $100/USgal, due to being taken overland several thousand miles through Pakistan under armed escort due to occasional Taliban attack.)
Industry uses toxic chemicals all the time. It's not a big deal. This is a chemical that's relatively easy to notice and where prolonged non-acute exposure doesn't have known harms. It's better than most.
Having said that, I'm still kind of excited. The basalt flood in Eastern Washington alone is in theory large enough to sequester hundreds of years of US emissions.
The 2nd sentence will eventually put it in a lower price range than fission.
When the world climate was 4.3 degrees Celsius colder, Boston was covered under a mile-high sheet of ice.
Lithification of CO2 (to make up a word?) is, as far as I know, endothermic. It takes energy to accomplish. On the surface, tending towards counter-productive. Burn fossil fuels to lithify CO2 from burning fossil fuels. Or ramp up nuclear, with all its problems, for the same.
Fusion, sure -- but we are not there, yet.
Unless we look at the sun -- solar and wind. (The largest fusion reactor we are going to have -- up in the sky.)
"Alternative", next-generation, "renewable" energy might allow us to divert part of its potential excess supply to lithification of CO2. At the "tailpipe/smokestack" of conventional production, or even, if we can figure out effective capture, out of the sky.
You want CO2 dealt with, you're going to need to find a way to package it into a stable solid state.
By the way, we already have one worldwide, extant system for lithification of CO2. Based upon solar energy. Photosynthesizing flora.
Trouble is, we are outracing its natural counterbalance while simultaneously reducing and eliminating the flora required for it.
Even if you somehow converted the gasses of Saturn into solids, the mass would result in a level of gravity that would not be survivable. I don't think there's any possibility for colonizing gas giants that doesn't involve something like Bespin or Jetsons floating platforms.
Both burn, and can be vaporized with LOX/acetyline torches:
http://www.popsci.com/sites/popsci.com/files/styles/medium_1...
But apparently, over long periods of time, and unless coerced, carbon prefers to be graphite and so, diamonds can decay as such. [0]
[0] https://en.wikipedia.org/wiki/Material_properties_of_diamond...
Hence why graphite is generally more plentiful than diamonds.
And you're talking about burning, not storage. Coal produces lots of dust and debris. I'm sure diamond would produce some dust at volumes.
https://www.quora.com/What-is-the-difference-between-coal-an...
Anyway, it's fantasy because I'm fairly confident we're not going to turn CO2 into mountains of diamonds in my lifetime!
Carbonate minerals are a lower energy compound than their reactants, which is good, because it means the reaction will happen spontaneously without an energy input from us (which would probably be too large to make it economical)
Then it becomes 1 CO2.
http://chemistry.elmhurst.edu/vchembook/511natgascombust.htm...
Can you get particulates burning methane? Long chain hydrocarbons, I can see how that works; but methane seems like it would disperse too easily, unless it's liquid/solid methane you're burning or you're doing it in a very low pressure atmosphere. That's my intuition though, any citations showing significant particulate yield with methane combustion?
I'm not sure what amounts of pollutants one would consider "significant". Certainly, gas turbines burning methane are comparatively low in pollutants, but even properly functioning automobile engines are extraordinarily low in pollutant emission (just for orientation, I don't consider CO2 "pollution").
http://www.gasturbine.org/images/thegasturbinesolution.pdf
https://www.enbridgegas.com/assets/docs/Gas%20Analysis%20Vic...
>gas turbines burning methane are comparatively low in pollutants //
Do they ever burn just methane or do they burn natural gas [that's been somewhat purified]?
I did have a search before posting and found citations claiming natural gas gave significant particulate reduction, as your second citation mentions, ergo the question of whether burning methane made any - it seems primarily to be a factor of burner efficiency, though there's research showing production of fullerenes and nanotubes that probably feeds in here too.
Looking further I found [1] which gives good info, in particular whilst gas:oil is 7:2704 in production of particulates by weight that citation notes that the PM2.5 [small particulates] as opposed to PM10 particulates may be significantly more damaging due to their penetration further in to the respitory system.
[1] http://www.eia.gov/pub/oil_gas/natural_gas/analysis_publicat...
Carbon storage may be a stop-gap but, as with "clean coal", is also used as a pr flag to justify continued fossil fuel expansion. With the price of solar dropping, that is where we should focus (and fusion).